You can restrict the use of Chrome to only the accounts you want to use it by enforcing a few group policies. The most recent of these is to force users to sign into Chrome. However, this policy need others to make it effective. Below are the ones I use.
Update - see this page for the latest policies that replace the first two listed below.
Firstly - force users to sign in to Chrome
Make sure they can only use a domain account
Update - see this page for the latest policies that replace the first two listed below.
Firstly - force users to sign in to Chrome
Make sure they can only use a domain account
Make sure they cannot use accounts you don't want them using in G Suite services
Disable incognito mode
Disable guest mode
Disable add user (might not want to use this for a staff account as they may need to use more than one account)
With this combination of policies, your users are locked down to their G Suite account and cannot do anything about it. Quick video on what it looks like:
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